Biofabrication of functional protein nanoparticles through simple His-tag engineering


Por: Lopez-Laguna, H, Sanchez, JM, Carratala, JV, Rojas-Pena, M, Sanchez-Garcia, L, Parlade, E, Sanchez-Chardi, A, Volta-Duran, E, Serna, N, Cano-Garrido, O, Flores, S, Ferrer-Miralles, N, Nolan, V, de Marco, A, Roher, N, Unzueta, U, Vazquez, E, Villaverde, A

Publicada: 13 sep 2021 Ahead of Print: 1 ago 2021
Resumen:
We have developed a simple, robust, and fully transversal approach for the a-la-carte fabrication of functional multimeric nanoparticles with potential biomedical applications, validated here by a set of diverse and unrelated polypeptides. The proposed concept is based on the controlled coordination between Zn2+ ions and His residues in His-tagged proteins. This approach results in a spontaneous and reproducible protein assembly as nanoscale oligomers that keep the original functionalities of the protein building blocks. The assembly of these materials is not linked to particular polypeptide features, and it is based on an environmentally friendly and sustainable approach. The resulting nanoparticles, with dimensions ranging between 10 and 15 nm, are regular in size, are architecturally stable, are fully functional, and serve as intermediates in a more complex assembly process, resulting in the formation of microscale protein materials. Since most of the recombinant proteins produced by biochemical and biotechnological industries and intended for biomedical research are His-tagged, the green biofabrication procedure proposed here can be straightforwardly applied to a huge spectrum of protein species for their conversion into their respective nanostructured formats.

Filiaciones:
Lopez-Laguna, H:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Sanchez, JM:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 Univ Nacl Cordoba, Fac Ciencias Exactas Fis & Nat, ICTA, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, Dept Quim, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, CONICET, Inst Invest Biol & Tecnoldg IIByT, RA-5016 Cordoba, Argentina

Carratala, JV:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Rojas-Pena, M:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

Sanchez-Garcia, L:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Parlade, E:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Sanchez-Chardi, A:
 Univ Autonoma Barcelona, Serv Microscopia, Barcelona 08193, Spain

 Univ Barcelona, Fac Biol, Dept Biol Evolut Ecol & Ciencies Ambientals, Barcelona 08028, Spain

Volta-Duran, E:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Serna, N:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

 Univ Autonoma Barcelona, Nanoligent SL, Edifici Eureka, Barcelona 08193, Spain

Cano-Garrido, O:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

 Univ Autonoma Barcelona, Nanoligent SL, OCG, Edifici Eureka, Barcelona 08193, Spain

Flores, S:
 Univ Nacl Cordoba, Fac Ciencias Exactas Fis & Nat, ICTA, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, Dept Quim, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, CONICET, Inst Invest Biol & Tecnoldg IIByT, RA-5016 Cordoba, Argentina

Ferrer-Miralles, N:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Nolan, V:
 Univ Nacl Cordoba, Fac Ciencias Exactas Fis & Nat, ICTA, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, Dept Quim, RA-5016 Cordoba, Argentina

 Univ Nacl Cordoba, CONICET, Inst Invest Biol & Tecnoldg IIByT, RA-5016 Cordoba, Argentina

de Marco, A:
 Univ Nova Gorica, Lab Environm & Life Sci, Nova Gorica 5000, Slovenia

Roher, N:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

 Univ Autonoma Barcelona, Dept Biol Cellular Fisiol Anim & Immunol, Barcelona 08193, Spain

Unzueta, U:
 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

 Biomed Res Inst St Pau IIB St Pau, Barcelona 08025, Spain

Vazquez, E:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain

Villaverde, A:
 Univ Autonoma Barcelona, Inst Biotecnol & Biomed, Barcelona 08193, Spain

 Univ Autonoma Barcelona, Dept Genet & Microbiol, Barcelona 08193, Spain

 CIBER Bioingn Biomat & Nanomed CIBER BBN, Madrid 28029, Spain
ISSN: 21680485
Editorial
AMER CHEMICAL SOC, 1155 16TH ST, NW, WASHINGTON, DC 20036 USA, Estados Unidos America
Tipo de documento: Article
Volumen: 9 Número: 36
Páginas: 12341-12354
WOS Id: 000696378200030
ID de PubMed: 34603855
imagen Green Published, hybrid

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